A numerical approach of interaction of methane thermocatalytic decomposition and microwave irradiation

Wei Hsin Chen, Hong Jyu Liou, Chen I. Hung

Research output: Contribution to journalArticle

7 Citations (Scopus)

Abstract

Thermocatalytic decomposition (TCD) of methane in association with microwave heating is a route to produce hydrogen without the formation of CO and CO2. To recognize the interaction characteristics of methane TCD and microwave irradiation in an activated carbon catalyst bed, the chemical reaction along with microwave-assisted heating is modeled and simulated numerically. The influences of microwave power, volumetric hourly space velocity (VHSV), and catalyst bed geometry on the performance of methane TCD are investigated. The predictions suggest that a higher microwave power can efficiently promote the performance. Increasing VHSV reduces CH4 conversion because of the lower residence time of methane in the catalyst bed; nevertheless, more hydrogen is produced. A smaller diameter of catalyst bed facilitates the chemical reaction. The distributions of temperature, reaction rate, and electric and magnetic fields in the catalyst bed at various operating conditions can be clearly observed. Consequently, the developed method and predictions are able to aid in figuring out the reaction phenomena of experimental work and designing the reactor for achieving methane TCD.

Original languageEnglish
Pages (from-to)13260-13271
Number of pages12
JournalInternational Journal of Hydrogen Energy
Volume38
Issue number30
DOIs
Publication statusPublished - 2013 Oct 8

All Science Journal Classification (ASJC) codes

  • Renewable Energy, Sustainability and the Environment
  • Fuel Technology
  • Condensed Matter Physics
  • Energy Engineering and Power Technology

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