TY - JOUR
T1 - Coexistence of magnetic and dielectric glassy states in alternating kagome and triangular lattice LuBaCo4 O7 cobaltite
AU - Dhanasekhar, C.
AU - Chandrasekhar Kakarla, D.
AU - Kumari, Archana
AU - Jawale, Monika
AU - Hindoddikar, Ronit
AU - Tiwari, Ajay
AU - Tirupathi, Patri
AU - Lai, Cang Ting
AU - Chou, Mitch M.C.
AU - Venimadhav, A.
AU - Yang, H. D.
AU - Chaddah, Praveen
AU - Mahajan, A. V.
N1 - Publisher Copyright:
© 2025 American Physical Society.
PY - 2025/5/1
Y1 - 2025/5/1
N2 - To date, the alternating kagome and triangular lattice cobaltites, i.e., RBaCo4O7 (R = Ca, Y, and rare-earth), have been well studied due to their large structural distortions, anisotropic exchange interactions, chiral spin liquid states, and giant multiferroic properties. Here, we report the coexistence of magnetic and dielectric glassy states in LuBaCo4O7 cobaltite below 50 K. AC magnetization studies show an absence of conventional spin freezing phenomena. The cooling and heating in unequal field (CHUF), thermal cycling of magnetization, and time-dependent magnetization studies at the low temperature (T) show the presence of the magnetic glassy state. The dielectric constant (ϵ′) exhibits a strong frequency-independent response at 45 K and dipolar glassy features below 20 K. The nonequilibrium magnetic glassy dynamics and dipolar glassy state at low T arises from the kinetic arrest of monoclinic (Cc) and orthorhombic (Pbn21) phases. From the dielectric probe, we are able to clearly distinguish the kinetically arrested phases at low T, whereas the bulk magnetization studies are unable to do so, as the arrested phases have low magnetic moments.
AB - To date, the alternating kagome and triangular lattice cobaltites, i.e., RBaCo4O7 (R = Ca, Y, and rare-earth), have been well studied due to their large structural distortions, anisotropic exchange interactions, chiral spin liquid states, and giant multiferroic properties. Here, we report the coexistence of magnetic and dielectric glassy states in LuBaCo4O7 cobaltite below 50 K. AC magnetization studies show an absence of conventional spin freezing phenomena. The cooling and heating in unequal field (CHUF), thermal cycling of magnetization, and time-dependent magnetization studies at the low temperature (T) show the presence of the magnetic glassy state. The dielectric constant (ϵ′) exhibits a strong frequency-independent response at 45 K and dipolar glassy features below 20 K. The nonequilibrium magnetic glassy dynamics and dipolar glassy state at low T arises from the kinetic arrest of monoclinic (Cc) and orthorhombic (Pbn21) phases. From the dielectric probe, we are able to clearly distinguish the kinetically arrested phases at low T, whereas the bulk magnetization studies are unable to do so, as the arrested phases have low magnetic moments.
UR - https://www.scopus.com/pages/publications/105005827645
UR - https://www.scopus.com/pages/publications/105005827645#tab=citedBy
U2 - 10.1103/PhysRevB.111.174438
DO - 10.1103/PhysRevB.111.174438
M3 - Article
AN - SCOPUS:105005827645
SN - 2469-9950
VL - 111
JO - Physical Review B
JF - Physical Review B
IS - 17
M1 - 174438
ER -