Effective transport properties accounting for electrochemical reactions of proton-exchange membrane fuel cell catalyst layers

Jon G. Pharoah, Hae Won Choi, Chih-Che Chueh, David B. Harvey

Research output: Chapter in Book/Report/Conference proceedingConference contribution

3 Citations (Scopus)

Abstract

There has been a rapidly growing interest in three-dimensional microstructural reconstruction of fuel cell electrodes so as to derive more accurate descriptors of the pertinent geometric and effective transport properties. Due to the limited accessibility of experiments based reconstruction techniques, such as dual-beam focused ion beamscanning electro microscopy or micro X-Ray computed tomography, within sample micro-structures of the catalyst layers in polymer electrolyte membrane fuel cells (PEMFCs), a particle based numerical model is used in this study to reconstruct sample microstructure of the catalyst layers in PEMFCs. Then the reconstructed sample structure is converted into the computational grid using body-fitted/cut-cell based unstructured meshing technique. Finally, finite volume methods (FVM) are applied to calculate effective properties on computational sample domains.

Original languageEnglish
Title of host publicationPolymer Electrolyte Fuel Cells 11
Pages221-227
Number of pages7
Edition1
DOIs
Publication statusPublished - 2011 Dec 1
Event11th Polymer Electrolyte Fuel Cell Symposium, PEFC 11 - 220th ECS Meeting - Boston, MA, United States
Duration: 2011 Oct 92011 Oct 14

Publication series

NameECS Transactions
Number1
Volume41
ISSN (Print)1938-5862
ISSN (Electronic)1938-6737

Other

Other11th Polymer Electrolyte Fuel Cell Symposium, PEFC 11 - 220th ECS Meeting
CountryUnited States
CityBoston, MA
Period11-10-0911-10-14

Fingerprint

Proton exchange membrane fuel cells (PEMFC)
Transport properties
Microstructure
Catalysts
Focused ion beams
Finite volume method
Tomography
Fuel cells
Numerical models
Microscopic examination
X rays
Electrodes
Experiments

All Science Journal Classification (ASJC) codes

  • Engineering(all)

Cite this

Pharoah, J. G., Choi, H. W., Chueh, C-C., & Harvey, D. B. (2011). Effective transport properties accounting for electrochemical reactions of proton-exchange membrane fuel cell catalyst layers. In Polymer Electrolyte Fuel Cells 11 (1 ed., pp. 221-227). (ECS Transactions; Vol. 41, No. 1). https://doi.org/10.1149/1.3635556
Pharoah, Jon G. ; Choi, Hae Won ; Chueh, Chih-Che ; Harvey, David B. / Effective transport properties accounting for electrochemical reactions of proton-exchange membrane fuel cell catalyst layers. Polymer Electrolyte Fuel Cells 11. 1. ed. 2011. pp. 221-227 (ECS Transactions; 1).
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Pharoah, JG, Choi, HW, Chueh, C-C & Harvey, DB 2011, Effective transport properties accounting for electrochemical reactions of proton-exchange membrane fuel cell catalyst layers. in Polymer Electrolyte Fuel Cells 11. 1 edn, ECS Transactions, no. 1, vol. 41, pp. 221-227, 11th Polymer Electrolyte Fuel Cell Symposium, PEFC 11 - 220th ECS Meeting, Boston, MA, United States, 11-10-09. https://doi.org/10.1149/1.3635556

Effective transport properties accounting for electrochemical reactions of proton-exchange membrane fuel cell catalyst layers. / Pharoah, Jon G.; Choi, Hae Won; Chueh, Chih-Che; Harvey, David B.

Polymer Electrolyte Fuel Cells 11. 1. ed. 2011. p. 221-227 (ECS Transactions; Vol. 41, No. 1).

Research output: Chapter in Book/Report/Conference proceedingConference contribution

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Pharoah JG, Choi HW, Chueh C-C, Harvey DB. Effective transport properties accounting for electrochemical reactions of proton-exchange membrane fuel cell catalyst layers. In Polymer Electrolyte Fuel Cells 11. 1 ed. 2011. p. 221-227. (ECS Transactions; 1). https://doi.org/10.1149/1.3635556