Electrochemical activity and durability of platinum nanoparticles supported on ordered mesoporous carbons for oxygen reduction reaction

Shou Heng Liu; Chien Chang Chiang; Min Tsung Wu; Shang Bin Liu

doi:10.1016/j.ijhydene.2009.12.183

Electrochemical activity and durability of platinum nanoparticles supported on ordered mesoporous carbons for oxygen reduction reaction

Shou Heng Liu, Chien Chang Chiang, Min Tsung Wu, Shang Bin Liu

Department of Environmental Engineering

Research output: Contribution to journal › Article › peer-review

57 Citations (Scopus)

Abstract

A facile procedure for synthesizing platinum nanoparticles (NPs) studded in ordered mesoporous carbons (Pt-OMCs) based on the organic-organic self-assembly (one-pot) approach is reported. These Pt-OMCs, which can be easily fabricated with controllable Pt loading, were found to possess high surface areas, highly accessible and stable active sites and superior electrocatalytic properties pertinent as cathode catalysts for hydrogen-oxygen fuel cells. The enhanced catalytic activity and durability observed for the Pt-OMC electrocatalysts are attributed to the strengthened interactions between the Pt catalyst and the mesoporous carbon that effectively precludes migration and/or agglomeration of Pt NPs on the carbon support.

Original language	English
Pages (from-to)	8149-8154
Number of pages	6
Journal	International Journal of Hydrogen Energy
Volume	35
Issue number	15
DOIs	https://doi.org/10.1016/j.ijhydene.2009.12.183
Publication status	Published - 2010 Aug

All Science Journal Classification (ASJC) codes

Renewable Energy, Sustainability and the Environment
Fuel Technology
Condensed Matter Physics
Energy Engineering and Power Technology

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1016/j.ijhydene.2009.12.183

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title = "Electrochemical activity and durability of platinum nanoparticles supported on ordered mesoporous carbons for oxygen reduction reaction",

abstract = "A facile procedure for synthesizing platinum nanoparticles (NPs) studded in ordered mesoporous carbons (Pt-OMCs) based on the organic-organic self-assembly (one-pot) approach is reported. These Pt-OMCs, which can be easily fabricated with controllable Pt loading, were found to possess high surface areas, highly accessible and stable active sites and superior electrocatalytic properties pertinent as cathode catalysts for hydrogen-oxygen fuel cells. The enhanced catalytic activity and durability observed for the Pt-OMC electrocatalysts are attributed to the strengthened interactions between the Pt catalyst and the mesoporous carbon that effectively precludes migration and/or agglomeration of Pt NPs on the carbon support.",

author = "Liu, {Shou Heng} and Chiang, {Chien Chang} and Wu, {Min Tsung} and Liu, {Shang Bin}",

note = "Funding Information: The supports of this work by the National Science Council , Taiwan ( NSC95-2113-M-001-040-MY3 and NSC98-2113-M-001-017-MY3 ) are gratefully acknowledged.",

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doi = "10.1016/j.ijhydene.2009.12.183",

language = "English",

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AU - Liu, Shou Heng

AU - Chiang, Chien Chang

AU - Wu, Min Tsung

AU - Liu, Shang Bin

N1 - Funding Information: The supports of this work by the National Science Council , Taiwan ( NSC95-2113-M-001-040-MY3 and NSC98-2113-M-001-017-MY3 ) are gratefully acknowledged.

PY - 2010/8

Y1 - 2010/8

N2 - A facile procedure for synthesizing platinum nanoparticles (NPs) studded in ordered mesoporous carbons (Pt-OMCs) based on the organic-organic self-assembly (one-pot) approach is reported. These Pt-OMCs, which can be easily fabricated with controllable Pt loading, were found to possess high surface areas, highly accessible and stable active sites and superior electrocatalytic properties pertinent as cathode catalysts for hydrogen-oxygen fuel cells. The enhanced catalytic activity and durability observed for the Pt-OMC electrocatalysts are attributed to the strengthened interactions between the Pt catalyst and the mesoporous carbon that effectively precludes migration and/or agglomeration of Pt NPs on the carbon support.

AB - A facile procedure for synthesizing platinum nanoparticles (NPs) studded in ordered mesoporous carbons (Pt-OMCs) based on the organic-organic self-assembly (one-pot) approach is reported. These Pt-OMCs, which can be easily fabricated with controllable Pt loading, were found to possess high surface areas, highly accessible and stable active sites and superior electrocatalytic properties pertinent as cathode catalysts for hydrogen-oxygen fuel cells. The enhanced catalytic activity and durability observed for the Pt-OMC electrocatalysts are attributed to the strengthened interactions between the Pt catalyst and the mesoporous carbon that effectively precludes migration and/or agglomeration of Pt NPs on the carbon support.

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JO - International Journal of Hydrogen Energy

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Electrochemical activity and durability of platinum nanoparticles supported on ordered mesoporous carbons for oxygen reduction reaction

Abstract

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