Enhanced charge carrier mobility in two-dimensional high dielectric molybdenum oxide

Sivacarendran Balendhran; Junkai Deng; Jian Zhen Ou; Sumeet Walia; James Scott; Jianshi Tang; Kang L. Wang; Matthew R. Field; Salvy Russo; Serge Zhuiykov; Michael S. Strano; Nikhil Medhekar; Sharath Sriram; Madhu Bhaskaran; Kourosh Kalantar-Zadeh

doi:10.1002/adma.201203346

Enhanced charge carrier mobility in two-dimensional high dielectric molybdenum oxide

Sivacarendran Balendhran, Junkai Deng, Jian Zhen Ou, Sumeet Walia, James Scott, Jianshi Tang, Kang L. Wang, Matthew R. Field, Salvy Russo, Serge Zhuiykov, Michael S. Strano, Nikhil Medhekar, Sharath Sriram, Madhu Bhaskaran, Kourosh Kalantar-Zadeh

College of Electrical Engineering and Computer Science

Research output: Contribution to journal › Article › peer-review

258 Citations (Scopus)

Abstract

We demonstrate that the energy bandgap of layered, high-dielectric α-MoO₃ can be reduced to values viable for the fabrication of 2D electronic devices. This is achieved through embedding Coulomb charges within the high dielectric media, advantageously limiting charge scattering. As a result, devices with α-MoO₃ of ∼11 nm thickness and carrier mobilities larger than 1100 cm² V^-1 s^-1 are obtained.

Original language	English
Pages (from-to)	109-114
Number of pages	6
Journal	Advanced Materials
Volume	25
Issue number	1
DOIs	https://doi.org/10.1002/adma.201203346
Publication status	Published - 2013 Jan 4

All Science Journal Classification (ASJC) codes

Materials Science(all)
Mechanics of Materials
Mechanical Engineering

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Balendhran, Sivacarendran ; Deng, Junkai ; Ou, Jian Zhen ; Walia, Sumeet ; Scott, James ; Tang, Jianshi ; Wang, Kang L. ; Field, Matthew R. ; Russo, Salvy ; Zhuiykov, Serge ; Strano, Michael S. ; Medhekar, Nikhil ; Sriram, Sharath ; Bhaskaran, Madhu ; Kalantar-Zadeh, Kourosh. / Enhanced charge carrier mobility in two-dimensional high dielectric molybdenum oxide. In: Advanced Materials. 2013 ; Vol. 25, No. 1. pp. 109-114.

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title = "Enhanced charge carrier mobility in two-dimensional high dielectric molybdenum oxide",

abstract = "We demonstrate that the energy bandgap of layered, high-dielectric α-MoO3 can be reduced to values viable for the fabrication of 2D electronic devices. This is achieved through embedding Coulomb charges within the high dielectric media, advantageously limiting charge scattering. As a result, devices with α-MoO3 of ∼11 nm thickness and carrier mobilities larger than 1100 cm2 V-1 s-1 are obtained.",

author = "Sivacarendran Balendhran and Junkai Deng and Ou, {Jian Zhen} and Sumeet Walia and James Scott and Jianshi Tang and Wang, {Kang L.} and Field, {Matthew R.} and Salvy Russo and Serge Zhuiykov and Strano, {Michael S.} and Nikhil Medhekar and Sharath Sriram and Madhu Bhaskaran and Kourosh Kalantar-Zadeh",

year = "2013",

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day = "4",

doi = "10.1002/adma.201203346",

language = "English",

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Enhanced charge carrier mobility in two-dimensional high dielectric molybdenum oxide. / Balendhran, Sivacarendran; Deng, Junkai; Ou, Jian Zhen; Walia, Sumeet; Scott, James; Tang, Jianshi; Wang, Kang L.; Field, Matthew R.; Russo, Salvy; Zhuiykov, Serge; Strano, Michael S.; Medhekar, Nikhil; Sriram, Sharath; Bhaskaran, Madhu; Kalantar-Zadeh, Kourosh.

In: Advanced Materials, Vol. 25, No. 1, 04.01.2013, p. 109-114.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Enhanced charge carrier mobility in two-dimensional high dielectric molybdenum oxide

AU - Balendhran, Sivacarendran

AU - Deng, Junkai

AU - Ou, Jian Zhen

AU - Walia, Sumeet

AU - Scott, James

AU - Tang, Jianshi

AU - Wang, Kang L.

AU - Field, Matthew R.

AU - Russo, Salvy

AU - Zhuiykov, Serge

AU - Strano, Michael S.

AU - Medhekar, Nikhil

AU - Sriram, Sharath

AU - Bhaskaran, Madhu

AU - Kalantar-Zadeh, Kourosh

PY - 2013/1/4

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AB - We demonstrate that the energy bandgap of layered, high-dielectric α-MoO3 can be reduced to values viable for the fabrication of 2D electronic devices. This is achieved through embedding Coulomb charges within the high dielectric media, advantageously limiting charge scattering. As a result, devices with α-MoO3 of ∼11 nm thickness and carrier mobilities larger than 1100 cm2 V-1 s-1 are obtained.

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JO - Advanced Materials

JF - Advanced Materials

SN - 0935-9648

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Enhanced charge carrier mobility in two-dimensional high dielectric molybdenum oxide

Abstract

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