High-stability transparent flexible energy storage based on PbZrO3/muscovite heterostructure

Deng Li Ko; Ti Hsin; Yu Hong Lai; Sheng Zhu Ho; Yunzhe Zheng; Rong Huang; Hao Pan; Yi Chun Chen; Ying Hao Chu

doi:10.1016/j.nanoen.2021.106149

High-stability transparent flexible energy storage based on PbZrO₃/muscovite heterostructure

Deng Li Ko, Ti Hsin, Yu Hong Lai, Sheng Zhu Ho, Yunzhe Zheng, Rong Huang, Hao Pan, Yi Chun Chen, Ying Hao Chu

Department of Physics

Research output: Contribution to journal › Review article › peer-review

21 Citations (Scopus)

Abstract

Antiferroelectric materials for dielectric energy storage with fast charging-discharging rate is an important research direction. In this study, to build a platform for the potential application in flexible transparent devices, a combination of the muscovite substrate and the antiferroelectric PbZrO₃ (PZO) is studied as a model system. The growth of PZO is first optimized on rigid substrates and then transferred to muscovite with the form of epitaxial and polycrystalline films. The energy storage performance with robust electrical and mechanical stability is systematically demonstrated. High energy densities of 46~52 J/cm³ were obtained; Compared with the epitaxial PZO, the polycrystalline PZO shows an increase of efficiency by 28% and possesses higher heat resistance. Moreover, fabricated on a transparent indium tin oxide electrode, the PZO heterostructure exhibits excellent energy performance and an optical transmittance of up to 70–80%. Through this study, a paradigm for reliable flexible transparent fast charging-discharging energy storage element is developed.

Original language	English
Article number	106149
Journal	Nano Energy
Volume	87
DOIs	https://doi.org/10.1016/j.nanoen.2021.106149
Publication status	Published - 2021 Sept

All Science Journal Classification (ASJC) codes

Renewable Energy, Sustainability and the Environment
Materials Science(all)
Electrical and Electronic Engineering

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10.1016/j.nanoen.2021.106149

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title = "High-stability transparent flexible energy storage based on PbZrO3/muscovite heterostructure",

abstract = "Antiferroelectric materials for dielectric energy storage with fast charging-discharging rate is an important research direction. In this study, to build a platform for the potential application in flexible transparent devices, a combination of the muscovite substrate and the antiferroelectric PbZrO3 (PZO) is studied as a model system. The growth of PZO is first optimized on rigid substrates and then transferred to muscovite with the form of epitaxial and polycrystalline films. The energy storage performance with robust electrical and mechanical stability is systematically demonstrated. High energy densities of 46~52 J/cm3 were obtained; Compared with the epitaxial PZO, the polycrystalline PZO shows an increase of efficiency by 28% and possesses higher heat resistance. Moreover, fabricated on a transparent indium tin oxide electrode, the PZO heterostructure exhibits excellent energy performance and an optical transmittance of up to 70–80%. Through this study, a paradigm for reliable flexible transparent fast charging-discharging energy storage element is developed.",

author = "Ko, {Deng Li} and Ti Hsin and Lai, {Yu Hong} and Ho, {Sheng Zhu} and Yunzhe Zheng and Rong Huang and Hao Pan and Chen, {Yi Chun} and Chu, {Ying Hao}",

note = "Funding Information: This work is supported by Ministry of Science and Technology, Taiwan (Grant Nos. MOST 106–2119-M-009–011-MY3 , 106–2628-E-009–001-MY2 , 106–2218-E-009–021 , 106–2923-M-009–003-MY2 , 107–2112-M-001–042-MY3 , 107–2218-E-007–050 ) and the Center for Emergent Functional Matter Science of National Yang Ming Chiao Tung University from The Featured Areas Research Center Program within the framework of the Higher Education Sprout Project by the Ministry of Education (MOE) in Taiwan. The work at East China Normal University was supported by the National Natural Science Foundation of China (Grant No. 61974042 ). Publisher Copyright: {\textcopyright} 2021 The Authors",

year = "2021",

month = sep,

doi = "10.1016/j.nanoen.2021.106149",

language = "English",

volume = "87",

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publisher = "Elsevier BV",

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T1 - High-stability transparent flexible energy storage based on PbZrO3/muscovite heterostructure

AU - Ko, Deng Li

AU - Hsin, Ti

AU - Lai, Yu Hong

AU - Ho, Sheng Zhu

AU - Zheng, Yunzhe

AU - Huang, Rong

AU - Pan, Hao

AU - Chen, Yi Chun

AU - Chu, Ying Hao

N1 - Funding Information: This work is supported by Ministry of Science and Technology, Taiwan (Grant Nos. MOST 106–2119-M-009–011-MY3 , 106–2628-E-009–001-MY2 , 106–2218-E-009–021 , 106–2923-M-009–003-MY2 , 107–2112-M-001–042-MY3 , 107–2218-E-007–050 ) and the Center for Emergent Functional Matter Science of National Yang Ming Chiao Tung University from The Featured Areas Research Center Program within the framework of the Higher Education Sprout Project by the Ministry of Education (MOE) in Taiwan. The work at East China Normal University was supported by the National Natural Science Foundation of China (Grant No. 61974042 ). Publisher Copyright: © 2021 The Authors

PY - 2021/9

Y1 - 2021/9

N2 - Antiferroelectric materials for dielectric energy storage with fast charging-discharging rate is an important research direction. In this study, to build a platform for the potential application in flexible transparent devices, a combination of the muscovite substrate and the antiferroelectric PbZrO3 (PZO) is studied as a model system. The growth of PZO is first optimized on rigid substrates and then transferred to muscovite with the form of epitaxial and polycrystalline films. The energy storage performance with robust electrical and mechanical stability is systematically demonstrated. High energy densities of 46~52 J/cm3 were obtained; Compared with the epitaxial PZO, the polycrystalline PZO shows an increase of efficiency by 28% and possesses higher heat resistance. Moreover, fabricated on a transparent indium tin oxide electrode, the PZO heterostructure exhibits excellent energy performance and an optical transmittance of up to 70–80%. Through this study, a paradigm for reliable flexible transparent fast charging-discharging energy storage element is developed.

AB - Antiferroelectric materials for dielectric energy storage with fast charging-discharging rate is an important research direction. In this study, to build a platform for the potential application in flexible transparent devices, a combination of the muscovite substrate and the antiferroelectric PbZrO3 (PZO) is studied as a model system. The growth of PZO is first optimized on rigid substrates and then transferred to muscovite with the form of epitaxial and polycrystalline films. The energy storage performance with robust electrical and mechanical stability is systematically demonstrated. High energy densities of 46~52 J/cm3 were obtained; Compared with the epitaxial PZO, the polycrystalline PZO shows an increase of efficiency by 28% and possesses higher heat resistance. Moreover, fabricated on a transparent indium tin oxide electrode, the PZO heterostructure exhibits excellent energy performance and an optical transmittance of up to 70–80%. Through this study, a paradigm for reliable flexible transparent fast charging-discharging energy storage element is developed.

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JO - Nano Energy

JF - Nano Energy

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ER -

High-stability transparent flexible energy storage based on PbZrO₃/muscovite heterostructure

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