Numerical analysis of transport and retardation for cesium in crushed granite using multi-stage advection–dispersion column experiments

Chuan Pin Lee; Ming Chee Wu; Shih Chin Tsai; Ching Yuan Liu; Tsuey Lin Tsai; Chun Hua Pan; Mon Shieh Yang

doi:10.1007/s10967-014-3888-1

Numerical analysis of transport and retardation for cesium in crushed granite using multi-stage advection–dispersion column experiments

Chuan Pin Lee, Ming Chee Wu, Shih Chin Tsai, Ching Yuan Liu, Tsuey Lin Tsai, Chun Hua Pan, Mon Shieh Yang

Department of Earth Sciences

Research output: Contribution to journal › Article

1 Citation (Scopus)

Abstract

In this study, a systematic analysis of cesium through crushed granite (0.297–0.840 mm) was constructed where synthetic groundwater and seawater were employed as the liquid phase. To build such models, multi-stage advection–dispersion column tests were conducted in order to determine the major transport processes and the calibration/validation of the hypothesized reactive transport models. The experimental breakthrough curves (BTCs) for HTO and Cs were both matched with their corresponding numerical BTCs by adjusting reaction and transport parameters such as forward or backward reaction rate constants (k_f or k_b), dispersivity (α), and porosity(θ).

Original language	English
Pages (from-to)	377-386
Number of pages	10
Journal	Journal of Radioanalytical and Nuclear Chemistry
Volume	304
Issue number	1
DOIs	https://doi.org/10.1007/s10967-014-3888-1
Publication status	Published - 2015 Apr 1

All Science Journal Classification (ASJC) codes

Analytical Chemistry
Nuclear Energy and Engineering
Radiology Nuclear Medicine and imaging
Pollution
Spectroscopy
Public Health, Environmental and Occupational Health
Health, Toxicology and Mutagenesis

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Lee, C. P., Wu, M. C., Tsai, S. C., Liu, C. Y., Tsai, T. L., Pan, C. H., & Yang, M. S. (2015). Numerical analysis of transport and retardation for cesium in crushed granite using multi-stage advection–dispersion column experiments. Journal of Radioanalytical and Nuclear Chemistry, 304(1), 377-386. https://doi.org/10.1007/s10967-014-3888-1

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abstract = "In this study, a systematic analysis of cesium through crushed granite (0.297–0.840 mm) was constructed where synthetic groundwater and seawater were employed as the liquid phase. To build such models, multi-stage advection–dispersion column tests were conducted in order to determine the major transport processes and the calibration/validation of the hypothesized reactive transport models. The experimental breakthrough curves (BTCs) for HTO and Cs were both matched with their corresponding numerical BTCs by adjusting reaction and transport parameters such as forward or backward reaction rate constants (kf or kb), dispersivity (α), and porosity(θ).",

author = "Lee, {Chuan Pin} and Wu, {Ming Chee} and Tsai, {Shih Chin} and Liu, {Ching Yuan} and Tsai, {Tsuey Lin} and Pan, {Chun Hua} and Yang, {Mon Shieh}",

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Numerical analysis of transport and retardation for cesium in crushed granite using multi-stage advection–dispersion column experiments. / Lee, Chuan Pin ; Wu, Ming Chee; Tsai, Shih Chin; Liu, Ching Yuan; Tsai, Tsuey Lin; Pan, Chun Hua; Yang, Mon Shieh.

In: Journal of Radioanalytical and Nuclear Chemistry, Vol. 304, No. 1, 01.04.2015, p. 377-386.

Research output: Contribution to journal › Article

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