TY - JOUR
T1 - Quantum critical behavior of the hyperkagome magnet Mn3CoSi
AU - Yamauchi, Hiroki
AU - Sari, Dita Puspita
AU - Yasui, Yukio
AU - Sakakura, Terutoshi
AU - Kimura, Hiroyuki
AU - Nakao, Akiko
AU - Ohhara, Takashi
AU - Honda, Takashi
AU - Kodama, Katsuaki
AU - Igawa, Naoki
AU - Ikeda, Kazutaka
AU - Iida, Kazuki
AU - Ueta, Daichi
AU - Yokoo, Tetsuya
AU - Frontzek, Matthias D.
AU - Chi, Songxue
AU - Fernandez-Baca, Jaime A.
AU - Kojima, Kenji M.
AU - Arseneau, Donald
AU - Morris, Gerald
AU - Hitti, Bassam
AU - Cai, Yipeng
AU - Berlie, Adam
AU - Watanabe, Isao
AU - Hsu, Pai Tse
AU - Chen, Yu Sheng
AU - Lee, Min Kai
AU - Hall, Amelia Elisabeth
AU - Balakrishnan, Geetha
AU - Chang, Lieh Jeng
AU - Shamoto, Shin Ichi
N1 - Publisher Copyright:
© 2024 authors. Published by the American Physical Society. Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.
PY - 2024/1
Y1 - 2024/1
N2 - β-Mn-type family alloys Mn3TX (T=Co, Rh, and Ir; X=Si and Ge) have a three-dimensional antiferromagnetic (AF) corner-shared triangular network, i.e., the hyperkagome lattice. The antiferromagnet Mn3RhSi shows magnetic short-range order over a wide temperature range of approximately 500 K above the Néel temperature TN of 190 K. In this family of compounds, as the lattice parameter decreases, the long-range magnetic ordering temperature decreases. Mn3CoSi has the smallest lattice parameter and the lowest TN in the family. The quantum critical point (QCP) from AF to the quantum paramagnetic state is expected near a cubic lattice parameter of 6.15 Å. Although the Néel temperature of Mn3CoSi is only 140 K, the emergence of the quantum critical behavior in Mn3CoSi is discussed. We study how the magnetic short-range order appears in Mn3CoSi by using neutron scattering, μSR, and bulk characterization such as specific heat capacity. According to the results, the neutron scattering intensity of the magnetic short-range order in Mn3CoSi does not change much at low temperatures from that of Mn3RhSi, although the μSR short-range order temperature of Mn3CoSi is largely suppressed to 240 K from that of Mn3RhSi. Correspondingly, the volume fraction of the magnetic short-range order regions, as shown by the initial asymmetry drop ratio of μSR above TN, also becomes small. Instead, the electronic-specific heat coefficient γ of Mn3CoSi is the largest in this Mn3TSi system, possibly due to the low-energy spin fluctuation near the quantum critical point.
AB - β-Mn-type family alloys Mn3TX (T=Co, Rh, and Ir; X=Si and Ge) have a three-dimensional antiferromagnetic (AF) corner-shared triangular network, i.e., the hyperkagome lattice. The antiferromagnet Mn3RhSi shows magnetic short-range order over a wide temperature range of approximately 500 K above the Néel temperature TN of 190 K. In this family of compounds, as the lattice parameter decreases, the long-range magnetic ordering temperature decreases. Mn3CoSi has the smallest lattice parameter and the lowest TN in the family. The quantum critical point (QCP) from AF to the quantum paramagnetic state is expected near a cubic lattice parameter of 6.15 Å. Although the Néel temperature of Mn3CoSi is only 140 K, the emergence of the quantum critical behavior in Mn3CoSi is discussed. We study how the magnetic short-range order appears in Mn3CoSi by using neutron scattering, μSR, and bulk characterization such as specific heat capacity. According to the results, the neutron scattering intensity of the magnetic short-range order in Mn3CoSi does not change much at low temperatures from that of Mn3RhSi, although the μSR short-range order temperature of Mn3CoSi is largely suppressed to 240 K from that of Mn3RhSi. Correspondingly, the volume fraction of the magnetic short-range order regions, as shown by the initial asymmetry drop ratio of μSR above TN, also becomes small. Instead, the electronic-specific heat coefficient γ of Mn3CoSi is the largest in this Mn3TSi system, possibly due to the low-energy spin fluctuation near the quantum critical point.
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U2 - 10.1103/PhysRevResearch.6.013144
DO - 10.1103/PhysRevResearch.6.013144
M3 - Article
AN - SCOPUS:85185182266
SN - 2643-1564
VL - 6
JO - Physical Review Research
JF - Physical Review Research
IS - 1
M1 - 013144
ER -