Upconversion Plasmonic Lasing from an Organolead Trihalide Perovskite Nanocrystal with Low Threshold

Yu Jung Lu, Teng Lam Shen, Kang Ning Peng, Pi Ju Cheng, Shu Wei Chang, Ming Yen Lu, Chih Wei Chu, Tzung Fang Guo, Harry A. Atwater

Research output: Contribution to journalArticlepeer-review

1 Citation (Scopus)

Abstract

The understanding of nonlinear light-matter interactions at the nanoscale has fueled worldwide interest in upconversion emission for imaging, lasing, and sensing. Upconversion lasers with anti-Stokes-type emission with various designs have been reported. However, reducing the volume and lasing threshold of such lasers to the nanoscale level is a fundamental photonics challenge. Here, we demonstrate that the upconversion efficiency can be improved by exploiting single-mode upconversion lasing from a single organo-lead halide perovskite nanocrystal in a resonance-adjustable plasmonic nanocavity. This upconversion plasmonic nanolaser has a very low lasing threshold (10 μJ cm-2) and a calculated ultrasmall mode volume (∼0.06 λ3) at 6 K. To provide the unique feature for lasing action, a temporal coherence signature of the upconversion plasmonic nanolasing was determined by measuring the second-order correlation function. The localized-electromagnetic-field confinement can be tailored in titanium nitride resonance-adjustable nanocavities, enhancing the pump-photon absorption and upconverted photon emission rate to achieve lasing. The proof-of-concept results significantly expand the performance of upconversion nanolasers, which are useful in applications such as on-chip, coherent, nonlinear optics, information processing, data storage, and sensing.

Original languageEnglish
Pages (from-to)335-342
Number of pages8
JournalACS Photonics
Volume8
Issue number1
DOIs
Publication statusPublished - 2021 Jan 20

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Biotechnology
  • Atomic and Molecular Physics, and Optics
  • Electrical and Electronic Engineering

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