Air-stable perovskite photovoltaic cells with low temperature deposited NiOx as an efficient hole-transporting material

A. K.Mahmud Hasan; Itaru Raifuku; N. Amin; Yasuaki Ishikawa; D. K. Sarkar; K. Sobayel; Mohammad R. Karim; Anwar Ul-Hamid; H. Abdullah; Md Shahiduzzaman; Yukiharu Uraoka; Kamaruzzaman Sopian; Md Akhtaruzzaman

doi:10.1364/OME.391321

Air-stable perovskite photovoltaic cells with low temperature deposited NiOx as an efficient hole-transporting material

A. K.Mahmud Hasan, Itaru Raifuku, N. Amin, Yasuaki Ishikawa, D. K. Sarkar, K. Sobayel, Mohammad R. Karim, Anwar Ul-Hamid, H. Abdullah, Md Shahiduzzaman, Yukiharu Uraoka, Kamaruzzaman Sopian, Md Akhtaruzzaman

光電科學與工程學系

研究成果: Article › 同行評審

1 引文斯高帕斯（Scopus）

摘要

The electron-beam physical vapor deposition (EBPVD) technique was selected for nickel oxide (NiOx) film deposition at room temperatures. NiOx film (18 nm thick) was deposited as a hole transporting material (HTM) for inverted perovskite solar cells (PSCs) onto a fluorine-doped tin oxide (FTO)-coated glass substrate at a chamber vacuum pressure of 4.6104 Pa. PSCs were fabricated as a glass/FTO/NiOx(HTM)/CH3NH3PbI3/PC61BM/BCP/Ag structure with as-deposited and annealed (500 °C for 30 min) NiOx films. Under 100 mW cm2 illumination, as-deposited and annealed NiOx as HTM in PSCs (0.16 cm2) showed a high-power conversion efficiency (PCE) of 13.20% and 13.24%, respectively. The as-deposited and annealed PSCs retained 72.2% and 76.96% of their initial efficiency in ambient conditions, correspondingly. This study highlights the possibility of achieving highly crystalline and finely disseminated NiOx films by EBPVD for fabricating efficient inverted PSCs.

原文	English
頁（從 - 到）	1801-1816
頁數	16
期刊	Optical Materials Express
卷	10
發行號	10
DOIs	https://doi.org/10.1364/OME.391321
出版狀態	Published - 2020 八月 1

All Science Journal Classification (ASJC) codes

Electronic, Optical and Magnetic Materials

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10.1364/OME.391321

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Hasan, A. K. M., Raifuku, I., Amin, N., Ishikawa, Y., Sarkar, D. K., Sobayel, K., Karim, M. R., Ul-Hamid, A., Abdullah, H., Shahiduzzaman, M., Uraoka, Y., Sopian, K., & Akhtaruzzaman, M. (2020). Air-stable perovskite photovoltaic cells with low temperature deposited NiOx as an efficient hole-transporting material. Optical Materials Express, 10(10), 1801-1816. https://doi.org/10.1364/OME.391321

Hasan, A. K.Mahmud ; Raifuku, Itaru ; Amin, N. ; Ishikawa, Yasuaki ; Sarkar, D. K. ; Sobayel, K. ; Karim, Mohammad R. ; Ul-Hamid, Anwar ; Abdullah, H. ; Shahiduzzaman, Md ; Uraoka, Yukiharu ; Sopian, Kamaruzzaman ; Akhtaruzzaman, Md. / Air-stable perovskite photovoltaic cells with low temperature deposited NiOx as an efficient hole-transporting material. 於: Optical Materials Express. 2020 ; 卷 10, 編號 10. 頁 1801-1816.

@article{34210712c391462595942e2670fdf512,

title = "Air-stable perovskite photovoltaic cells with low temperature deposited NiOx as an efficient hole-transporting material",

abstract = "The electron-beam physical vapor deposition (EBPVD) technique was selected for nickel oxide (NiOx) film deposition at room temperatures. NiOx film (18 nm thick) was deposited as a hole transporting material (HTM) for inverted perovskite solar cells (PSCs) onto a fluorine-doped tin oxide (FTO)-coated glass substrate at a chamber vacuum pressure of 4.6104 Pa. PSCs were fabricated as a glass/FTO/NiOx(HTM)/CH3NH3PbI3/PC61BM/BCP/Ag structure with as-deposited and annealed (500 °C for 30 min) NiOx films. Under 100 mW cm2 illumination, as-deposited and annealed NiOx as HTM in PSCs (0.16 cm2) showed a high-power conversion efficiency (PCE) of 13.20% and 13.24%, respectively. The as-deposited and annealed PSCs retained 72.2% and 76.96% of their initial efficiency in ambient conditions, correspondingly. This study highlights the possibility of achieving highly crystalline and finely disseminated NiOx films by EBPVD for fabricating efficient inverted PSCs.",

author = "Hasan, {A. K.Mahmud} and Itaru Raifuku and N. Amin and Yasuaki Ishikawa and Sarkar, {D. K.} and K. Sobayel and Karim, {Mohammad R.} and Anwar Ul-Hamid and H. Abdullah and Md Shahiduzzaman and Yukiharu Uraoka and Kamaruzzaman Sopian and Md Akhtaruzzaman",

note = "Funding Information: Universiti Kebangsaan Malaysia (LRGS/1/2019/UKM-UKM/6/1). The authors would like to acknowledge the Long Term Research Grant Scheme (LRGS) (LRGS/1/2019/UKM-UKM/6/1) grant funded by the University Kebangsaan Malaysia.",

year = "2020",

month = aug,

day = "1",

doi = "10.1364/OME.391321",

language = "English",

volume = "10",

pages = "1801--1816",

journal = "Optical Materials Express",

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Hasan, AKM, Raifuku, I, Amin, N, Ishikawa, Y, Sarkar, DK, Sobayel, K, Karim, MR, Ul-Hamid, A, Abdullah, H, Shahiduzzaman, M, Uraoka, Y, Sopian, K & Akhtaruzzaman, M 2020, 'Air-stable perovskite photovoltaic cells with low temperature deposited NiOx as an efficient hole-transporting material', Optical Materials Express, 卷 10, 編號 10, 頁 1801-1816. https://doi.org/10.1364/OME.391321

Air-stable perovskite photovoltaic cells with low temperature deposited NiOx as an efficient hole-transporting material. / Hasan, A. K.Mahmud; Raifuku, Itaru; Amin, N.; Ishikawa, Yasuaki; Sarkar, D. K.; Sobayel, K.; Karim, Mohammad R.; Ul-Hamid, Anwar; Abdullah, H.; Shahiduzzaman, Md; Uraoka, Yukiharu; Sopian, Kamaruzzaman; Akhtaruzzaman, Md.

於: Optical Materials Express, 卷 10, 編號 10, 01.08.2020, p. 1801-1816.

研究成果: Article › 同行評審

TY - JOUR

T1 - Air-stable perovskite photovoltaic cells with low temperature deposited NiOx as an efficient hole-transporting material

AU - Hasan, A. K.Mahmud

AU - Raifuku, Itaru

AU - Amin, N.

AU - Ishikawa, Yasuaki

AU - Sarkar, D. K.

AU - Sobayel, K.

AU - Karim, Mohammad R.

AU - Ul-Hamid, Anwar

AU - Abdullah, H.

AU - Shahiduzzaman, Md

AU - Uraoka, Yukiharu

AU - Sopian, Kamaruzzaman

AU - Akhtaruzzaman, Md

N1 - Funding Information: Universiti Kebangsaan Malaysia (LRGS/1/2019/UKM-UKM/6/1). The authors would like to acknowledge the Long Term Research Grant Scheme (LRGS) (LRGS/1/2019/UKM-UKM/6/1) grant funded by the University Kebangsaan Malaysia.

PY - 2020/8/1

Y1 - 2020/8/1

N2 - The electron-beam physical vapor deposition (EBPVD) technique was selected for nickel oxide (NiOx) film deposition at room temperatures. NiOx film (18 nm thick) was deposited as a hole transporting material (HTM) for inverted perovskite solar cells (PSCs) onto a fluorine-doped tin oxide (FTO)-coated glass substrate at a chamber vacuum pressure of 4.6104 Pa. PSCs were fabricated as a glass/FTO/NiOx(HTM)/CH3NH3PbI3/PC61BM/BCP/Ag structure with as-deposited and annealed (500 °C for 30 min) NiOx films. Under 100 mW cm2 illumination, as-deposited and annealed NiOx as HTM in PSCs (0.16 cm2) showed a high-power conversion efficiency (PCE) of 13.20% and 13.24%, respectively. The as-deposited and annealed PSCs retained 72.2% and 76.96% of their initial efficiency in ambient conditions, correspondingly. This study highlights the possibility of achieving highly crystalline and finely disseminated NiOx films by EBPVD for fabricating efficient inverted PSCs.

AB - The electron-beam physical vapor deposition (EBPVD) technique was selected for nickel oxide (NiOx) film deposition at room temperatures. NiOx film (18 nm thick) was deposited as a hole transporting material (HTM) for inverted perovskite solar cells (PSCs) onto a fluorine-doped tin oxide (FTO)-coated glass substrate at a chamber vacuum pressure of 4.6104 Pa. PSCs were fabricated as a glass/FTO/NiOx(HTM)/CH3NH3PbI3/PC61BM/BCP/Ag structure with as-deposited and annealed (500 °C for 30 min) NiOx films. Under 100 mW cm2 illumination, as-deposited and annealed NiOx as HTM in PSCs (0.16 cm2) showed a high-power conversion efficiency (PCE) of 13.20% and 13.24%, respectively. The as-deposited and annealed PSCs retained 72.2% and 76.96% of their initial efficiency in ambient conditions, correspondingly. This study highlights the possibility of achieving highly crystalline and finely disseminated NiOx films by EBPVD for fabricating efficient inverted PSCs.

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