CO Electroreduction: Current Development and Understanding of Cu-Based Catalysts

Haochen Zhang, Jing Li, Mu Jeng Cheng, Qi Lu

研究成果: Article

6 引文 (Scopus)

摘要

Electrochemical synthesis of value-added chemicals from CO and H 2 O powered by renewable energy is a promising technique to supplement, if not eventually replace, the Fischer-Tropsch process, which requires high energy input (i.e., typical temperatures of 200-400 °C and pressures of 10-200 atm) and large-scale reactors that are difficult to match to the disperse renewable energy sources. Moreover, this technique is also ideal for implementing the electroreduction of CO 2 using a tandem strategy because many catalysts can convert CO 2 to CO with high efficiency. However, the direct reduction of CO 2 to more valuable hydrocarbons and oxygenates is hindered by the lack of efficient catalysts. This perspective highlights the current understanding and progress of CO electroreduction from both experimental and computational approaches. The challenges that must be overcome for further development are also identified and discussed.

原文English
頁(從 - 到)49-65
頁數17
期刊ACS Catalysis
9
發行號1
DOIs
出版狀態Published - 2019 一月 4

指紋

Carbon Monoxide
Catalysts
Hydrocarbons
Temperature

All Science Journal Classification (ASJC) codes

  • Catalysis
  • Chemistry(all)

引用此文

Zhang, Haochen ; Li, Jing ; Cheng, Mu Jeng ; Lu, Qi. / CO Electroreduction : Current Development and Understanding of Cu-Based Catalysts. 於: ACS Catalysis. 2019 ; 卷 9, 編號 1. 頁 49-65.
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CO Electroreduction : Current Development and Understanding of Cu-Based Catalysts. / Zhang, Haochen; Li, Jing; Cheng, Mu Jeng; Lu, Qi.

於: ACS Catalysis, 卷 9, 編號 1, 04.01.2019, p. 49-65.

研究成果: Article

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