Cobalt Catalysts Derived from Layered Double Hydroxide/g-C3N4 Composite in the Hydrogenation of γ-Valerolactone into 1,4-Pentanediol

Yu Chuan Lin; Chou Hsun Hsieh

doi:10.1007/s10563-022-09383-7

Cobalt Catalysts Derived from Layered Double Hydroxide/g-C₃N₄ Composite in the Hydrogenation of γ-Valerolactone into 1,4-Pentanediol

Yu Chuan Lin
, Chou Hsun Hsieh

化學工程學系

研究成果: Article › 同行評審

2 引文斯高帕斯（Scopus）

摘要

Co-based catalysts were derived from CoAl-layered double hydroxide (LDH), LDH/melamine, LDH/activated carbon, and LDH/g-C₃N₄. The use of these catalysts for the hydrogenation of γ-valerolactone into 1,4-pentanediol was investigated. The catalyst derived from CoAl-LDH/g-C₃N₄ contained higher concentrations of strong Brønsted acid, Lewis acid (Co^δ+, δ > 2), and Lewis base (N with a lone pair of electrons) sites, resulting in improved turnover frequency.

原文	English
頁（從 - 到）	20-28
頁數	9
期刊	Catalysis Surveys from Asia
卷	27
發行號	1
DOIs	https://doi.org/10.1007/s10563-022-09383-7
出版狀態	Published - 2023 3月

All Science Journal Classification (ASJC) codes

催化
一般化學

存取文件

10.1007/s10563-022-09383-7

其它文件與鏈接

引用此

@article{215aa4bd413044f89dcc881a6154fea1,

title = "Cobalt Catalysts Derived from Layered Double Hydroxide/g-C3N4 Composite in the Hydrogenation of γ-Valerolactone into 1,4-Pentanediol",

abstract = "Co-based catalysts were derived from CoAl-layered double hydroxide (LDH), LDH/melamine, LDH/activated carbon, and LDH/g-C3N4. The use of these catalysts for the hydrogenation of γ-valerolactone into 1,4-pentanediol was investigated. The catalyst derived from CoAl-LDH/g-C3N4 contained higher concentrations of strong Br{\o}nsted acid, Lewis acid (Coδ+, δ > 2), and Lewis base (N with a lone pair of electrons) sites, resulting in improved turnover frequency.",

author = "Lin, \{Yu Chuan\} and Hsieh, \{Chou Hsun\}",

note = "Publisher Copyright: {\textcopyright} 2022, The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature.",

year = "2023",

month = mar,

doi = "10.1007/s10563-022-09383-7",

language = "English",

volume = "27",

pages = "20--28",

journal = "Catalysis Surveys from Asia",

issn = "1571-1013",

publisher = "Springer",

number = "1",

}

TY - JOUR

T1 - Cobalt Catalysts Derived from Layered Double Hydroxide/g-C3N4 Composite in the Hydrogenation of γ-Valerolactone into 1,4-Pentanediol

AU - Lin, Yu Chuan

AU - Hsieh, Chou Hsun

PY - 2023/3

Y1 - 2023/3

N2 - Co-based catalysts were derived from CoAl-layered double hydroxide (LDH), LDH/melamine, LDH/activated carbon, and LDH/g-C3N4. The use of these catalysts for the hydrogenation of γ-valerolactone into 1,4-pentanediol was investigated. The catalyst derived from CoAl-LDH/g-C3N4 contained higher concentrations of strong Brønsted acid, Lewis acid (Coδ+, δ > 2), and Lewis base (N with a lone pair of electrons) sites, resulting in improved turnover frequency.

AB - Co-based catalysts were derived from CoAl-layered double hydroxide (LDH), LDH/melamine, LDH/activated carbon, and LDH/g-C3N4. The use of these catalysts for the hydrogenation of γ-valerolactone into 1,4-pentanediol was investigated. The catalyst derived from CoAl-LDH/g-C3N4 contained higher concentrations of strong Brønsted acid, Lewis acid (Coδ+, δ > 2), and Lewis base (N with a lone pair of electrons) sites, resulting in improved turnover frequency.

UR - https://www.scopus.com/pages/publications/85141751233

UR - https://www.scopus.com/pages/publications/85141751233#tab=citedBy

U2 - 10.1007/s10563-022-09383-7

DO - 10.1007/s10563-022-09383-7

M3 - Article

AN - SCOPUS:85141751233

SN - 1571-1013

VL - 27

SP - 20

EP - 28

JO - Catalysis Surveys from Asia

JF - Catalysis Surveys from Asia

IS - 1

ER -

Cobalt Catalysts Derived from Layered Double Hydroxide/g-C3N4 Composite in the Hydrogenation of γ-Valerolactone into 1,4-Pentanediol

摘要

All Science Journal Classification (ASJC) codes

存取文件

其它文件與鏈接

指紋

引用此

Cobalt Catalysts Derived from Layered Double Hydroxide/g-C₃N₄ Composite in the Hydrogenation of γ-Valerolactone into 1,4-Pentanediol