TY - JOUR
T1 - Correlation-driven electronic nematicity in the Dirac semimetal BaNiS2
AU - Butler, Christopher John
AU - Kohsaka, Yuhki
AU - Yamakawa, Youichi
AU - Bahramy, Mohammad Saeed
AU - Onari, Seiichiro
AU - Kontani, Hiroshi
AU - Hanaguri, Tetsuo
AU - Shamoto, Shinichi
N1 - Funding Information:
ACKNOWLEDGMENTS. We are grateful to T. Machida and A. Gauzzi for helpful discussions. This work was supported by JST CREST Grant No. JPMJCR16F2, and by a Grant-in-Aid for Scientific Research on Innovative Areas “Quantum Liquid Crystals” (KAKENHI Grant No. JP19H05824 and No. JP19H05825) from JSPS of Japan. C.J.B. acknowledges support from RIKEN’s Programs for Junior Scientists.
Publisher Copyright:
Copyright © 2022 the Author(s). Published by PNAS. This open access article is distributed under Creative Commons Attribution License 4.0 (CC BY).
PY - 2022/12/6
Y1 - 2022/12/6
N2 - In BaNiS2, a Dirac nodal line band structure exists within a two-dimensional Ni square lattice system, in which significant electronic correlation effects are anticipated. Using scanning tunneling microscopy (STM), we discover signs of correlated-electron behavior, namely electronic nematicity appearing as a pair of C2-symmetry striped patterns in the local density-of-states at ∼60 meV above the Fermi energy. In observations of quasiparticle interference, as well as identifying scattering between Dirac cones, we find that the striped patterns in real space stem from a lifting of degeneracy among electron pockets at the Brillouin zone boundary. We infer a momentum-dependent energy shift with d-form factor, which we model numerically within a density wave (DW) equation framework that considers spin-fluctuation-driven nematicity. This suggests an unusual mechanism driving the nematic instability, stemming from only a small perturbation to the Fermi surface, in a system with very low density of states at the Fermi energy. The Dirac points lie at nodes of the d-form factor and are almost unaffected by it. These results highlight BaNiS2 as a unique material in which Dirac electrons and symmetry-breaking electronic correlations coexist.
AB - In BaNiS2, a Dirac nodal line band structure exists within a two-dimensional Ni square lattice system, in which significant electronic correlation effects are anticipated. Using scanning tunneling microscopy (STM), we discover signs of correlated-electron behavior, namely electronic nematicity appearing as a pair of C2-symmetry striped patterns in the local density-of-states at ∼60 meV above the Fermi energy. In observations of quasiparticle interference, as well as identifying scattering between Dirac cones, we find that the striped patterns in real space stem from a lifting of degeneracy among electron pockets at the Brillouin zone boundary. We infer a momentum-dependent energy shift with d-form factor, which we model numerically within a density wave (DW) equation framework that considers spin-fluctuation-driven nematicity. This suggests an unusual mechanism driving the nematic instability, stemming from only a small perturbation to the Fermi surface, in a system with very low density of states at the Fermi energy. The Dirac points lie at nodes of the d-form factor and are almost unaffected by it. These results highlight BaNiS2 as a unique material in which Dirac electrons and symmetry-breaking electronic correlations coexist.
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U2 - 10.1073/pnas.2212730119
DO - 10.1073/pnas.2212730119
M3 - Article
C2 - 36459647
AN - SCOPUS:85143460797
SN - 0027-8424
VL - 119
JO - Proceedings of the National Academy of Sciences of the United States of America
JF - Proceedings of the National Academy of Sciences of the United States of America
IS - 49
M1 - e2212730119
ER -