Firefly-like water splitting cells based on FRET phenomena with ultrahigh performance over 12%

Yi Sheng Lai, Fei Pan, Yen Hsun Su

研究成果: Article同行評審

3 引文 斯高帕斯(Scopus)

摘要

A firefly-like chemiluminescence reaction was utilized in a ZrO2 nanoparticle matrix of water splitting cells, where the chlorophyll of Lantana camara was used as the major photosensitizer to excite electrons to the conduction band of ZrO2. The fluorescence resonance energy transfer (FRET) was induced by rubrene, a firefly-like chemiluminescence molecule, and Lantana camara chlorophyll combined with 9,10-diphenylanthracene. The ZrO2 nanoparticle film coated by the chlorophyll of Lantana camara and 9,10-diphenylanthracene under chemiluminescence irradiation in 1 M KHCO3 water solution demonstrated the highest photocurrent density (88.1 A/m2) and the highest water splitting efficiency (12.77%).

原文English
頁(從 - 到)5007-5013
頁數7
期刊ACS Applied Materials and Interfaces
10
發行號5
DOIs
出版狀態Published - 2018 一月 1

All Science Journal Classification (ASJC) codes

  • Materials Science(all)

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