Low-carrier density and fragile magnetism in a Kondo lattice system

Binod K. Rai, Iain W.H. Oswald, Wenjing Ban, C. L. Huang, V. Loganathan, A. M. Hallas, M. N. Wilson, G. M. Luke, L. Harriger, Q. Huang, Y. Li, Sami Dzsaber, Julia Y. Chan, N. L. Wang, Silke Paschen, J. W. Lynn, Andriy H. Nevidomskyy, Pengcheng Dai, Q. Si, E. Morosan

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4 引文 斯高帕斯(Scopus)

摘要

Kondo-based semimetals and semiconductors are of extensive current interest as a viable platform for strongly correlated states in the dilute carrier limit. It is thus important to explore the routes to understand such systems. One established pathway is through the Kondo effect in metallic nonmagnetic analogs, in the so called half-filling case of one conduction electron and one 4f electron per site. Here, we demonstrate that Kondo-based semimetals develop out of conduction electrons with a low-carrier density in the presence of an even number of rare-earth sites. We do so by studying the Kondo material Yb3Ir4Ge13 along with its closed-4f-shell counterpart, Lu3Ir4Ge13. Through magnetotransport, optical conductivity, and thermodynamic measurements, we establish that the correlated semimetallic state of Yb3Ir4Ge13 below its Kondo temperature originates from the Kondo effect of a low-carrier conduction-electron background. In addition, it displays fragile magnetism at very low temperatures, which in turn, can be tuned to a Griffiths-phase-like regime through Lu-for-Yb substitution. These findings are connected with recent theoretical studies in simplified models. Our results can pave the way to exploring strong correlation physics in a semimetallic environment.

原文English
文章編號085120
期刊Physical Review B
99
發行號8
DOIs
出版狀態Published - 2019 二月 12

All Science Journal Classification (ASJC) codes

  • 電子、光磁材料
  • 凝聚態物理學

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