TY - JOUR
T1 - Magnetic excitations in the ground state of Yb 2 Ti 2 O 7
AU - Peçanha-Antonio, Viviane
AU - Feng, Erxi
AU - Su, Yixi
AU - Pomjakushin, Vladimir
AU - Demmel, Franz
AU - Chang, Lieh Jeng
AU - Aldus, Robert J.
AU - Xiao, Yinguo
AU - Lees, Martin R.
AU - Brückel, Thomas
N1 - Publisher Copyright:
© 2017 American Physical Society.
PY - 2017/12/11
Y1 - 2017/12/11
N2 - We report an extensive study on the zero field ground state of a powder sample of the pyrochlore Yb 2 Ti 2 O 7 . A sharp heat capacity anomaly that labels a low temperature phase transition in this material is observed at 280 mK. Neutron diffraction shows that a quasicollinear ferromagnetic order develops below Tc with a magnetic moment of 0.87(2)μB. High resolution inelastic neutron scattering measurements show, below the phase transition temperature, sharp gapped low-lying magnetic excitations coexisting with a remnant quasielastic contribution likely associated with persistent spin fluctuations. Moreover, a broad inelastic continuum of excitations at ∼0.6 meV is observed from the lowest measured temperature up to at least 2.5 K. At 10 K, the continuum has vanished and a broad quasielastic conventional paramagnetic scattering takes place at the observed energy range. Finally, we show that the exchange parameters obtained within the framework of linear spin-wave theory do not accurately describe the observed zero field inelastic neutron scattering data.
AB - We report an extensive study on the zero field ground state of a powder sample of the pyrochlore Yb 2 Ti 2 O 7 . A sharp heat capacity anomaly that labels a low temperature phase transition in this material is observed at 280 mK. Neutron diffraction shows that a quasicollinear ferromagnetic order develops below Tc with a magnetic moment of 0.87(2)μB. High resolution inelastic neutron scattering measurements show, below the phase transition temperature, sharp gapped low-lying magnetic excitations coexisting with a remnant quasielastic contribution likely associated with persistent spin fluctuations. Moreover, a broad inelastic continuum of excitations at ∼0.6 meV is observed from the lowest measured temperature up to at least 2.5 K. At 10 K, the continuum has vanished and a broad quasielastic conventional paramagnetic scattering takes place at the observed energy range. Finally, we show that the exchange parameters obtained within the framework of linear spin-wave theory do not accurately describe the observed zero field inelastic neutron scattering data.
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U2 - 10.1103/PhysRevB.96.214415
DO - 10.1103/PhysRevB.96.214415
M3 - Article
AN - SCOPUS:85039446633
SN - 2469-9950
VL - 96
JO - Physical Review B
JF - Physical Review B
IS - 21
M1 - 214415
ER -