Modulating the line shape of magnetoconductance by varying the charge injection in polymer light-emitting diodes

Nidya Chitraningrum, Ting Yi Chu, Ping Tsung Huang, Ten Chin Wen, Tzung Fang Guo

研究成果: Article同行評審

2 引文 斯高帕斯(Scopus)

摘要

We fabricate the phenyl-substituted poly(p-phenylene vinylene) copolymer (super yellow, SY-PPV)-based polymer light-emitting diodes (PLEDs) with different device architectures to modulate the injection of opposite charge carriers and investigate the corresponding magnetoconductance (MC) responses. At the first glance, we find that all PLEDs exhibit the positive MC responses. By applying the mathematical analysis to fit the curves with two empirical equations of a non-Lorentzian and a Lorentzian function, we are able to extract the hidden negative MC component from the positive MC curve. We attribute the growth of the negative MC component to the reduced interaction of the triplet excitons with charges to generate the free charge carriers as modulated by the applied magnetic field, known as the triplet exciton-charge reaction, by analyzing MC responses for PLEDs of the charge-unbalanced and hole-blocking device configurations. The negative MC component causes the broadening of the line shape in MC curves.

原文English
文章編號025209
期刊AIP Advances
8
發行號2
DOIs
出版狀態Published - 2018 二月 1

All Science Journal Classification (ASJC) codes

  • 物理與天文學 (全部)

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