The emission and distribution of PCDD/Fs in municipal solid waste incinerators and coal-fired power plant

Wen Yinn Lin, Yee Lin Wu, Li Kai Tu, Lin Chi Wang, Xin Lu

研究成果: Article同行評審

46 引文 斯高帕斯(Scopus)

摘要

The emission and distribution of polychlorinated debenzo-p-dioxins/dibenzofurans (PCDD/Fs) was investigated in two municipal solid waste incinerators (MSWIs) and one coal-fired power plant (PP) in southern Taiwan. Samples were collected from stack flue gases (SFG), bottom residues (BR), super heater (SH), economizer (EC), semi-dry absorber (SDA), bag filter (BF), and fly ash pit (FAP) in MSWIs. Stack flue gases, bottom residues and electrostatic dust collectors (ESD) in PP were also collected. In order to compare the difference between the results of MSWIs and PP, samples from SFG, BS, and FAP in a PP were also determined. Seventeen congeners of PCDD/Fs were analyzed by utilizing a high-resolution gas chromatograph/high-resolution mass spectrometer (HRGC/HRMS). Distributions of total PCDD/F-I-TEQ in each unit of MSWI-A and MSWI-B were SFG (0.3%, 0.07%), BR (3.9%, 0.62%), SH (0.17%, 0.24%), EC (4.2%, 0.05%), SDA (1.29%, 7.06%), and BF (90.14%, 91.97%), respectively. However, those in SFG, BS, and FAP of PP were 99.58%, 0.17%, and 0.25%, respectively. The above results indicated 99.5% PCDD/Fs were trapped in the fly ash of MWSI. On the other hand, 99.7% PCDD/Fs was emitted to the atmosphere from PP. The results of this study provide useful information for controlling PCDD/Fs in MSWIs and PP.

原文English
頁(從 - 到)519-532
頁數14
期刊Aerosol and Air Quality Research
10
發行號6
DOIs
出版狀態Published - 2010 12月

All Science Journal Classification (ASJC) codes

  • 環境化學
  • 污染

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