The temperature evolution of the magnetic correlations in pure and diluted spin ice Ho2-xYxTi2O7

L. J. Chang, Y. Su, Y. J. Kao, Y. Z. Chou, K. Kakurai, R. Mittal, H. Schneider, Th Brückel, G. Balakrishnan, M. R. Lees

研究成果: Article同行評審

1 引文 斯高帕斯(Scopus)


Diffuse polarized neutron scattering studies have been carried out on single crystals of pyrochlore spin ice Ho2-xYxTi 2O7 (x=0, 0.3, and 1) to investigate the effects of doping and anisotropy on spin correlations in the system. The crystals were aligned with the (1 -1 0) orientation coincident with the direction of neutron polarization. For all the samples studied the spin flip (SF) diffuse scattering (i.e. the in-plane component) reveals that the spin correlations can be described using a nearest-neighbour spin ice model (NNSM) at higher temperatures (T=3.6 K) and a dipolar spin ice model (DSM) as the temperature is reduced (T=30 mK). In the non-spin flip (NSF) channel (i.e. the out-of-plane component), the signature of strong antiferromagnetic correlations is observed for all the samples at the same temperature as the dipolar spin ice behaviour appears in the SF channel. Our studies show that the non-magnetic dopant Y does not significantly alter SF or NSF scattering for the spin ice state, even when Y doping is as high as 50%. In this paper, we focus on the experimental results of the highly doped spin ice HoYTi2O7 and compare our results with pure spin ice Ho2Ti2O7. The crossover from a dipolar to a nearest-neighbour spin ice behaviour and the doping insensitivity in spin ices are briefly discussed.

頁(從 - 到)2393-2396
期刊Physica B: Condensed Matter
出版狀態Published - 2011 六月

All Science Journal Classification (ASJC) codes

  • 電子、光磁材料
  • 凝聚態物理學
  • 電氣與電子工程


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